Kinetically assisted potential sputtering of insulators by highly charged ions; ; et al in Physical Review Letters (2001), 86(16), 3530-3533 A new form of potential sputtering has been found for impact of slow (less than or equal to 1500 eV) multiply charged Xe ions (charge states up to q = 25) on MgOx. In contrast to alkali-halide or SiO2 ... [more ▼] A new form of potential sputtering has been found for impact of slow (less than or equal to 1500 eV) multiply charged Xe ions (charge states up to q = 25) on MgOx. In contrast to alkali-halide or SiO2 surfaces this mechanism requires the simultaneous presence of electronic excitation of the target material and of a kinetically formed collision cascade within the target in order to initiate the sputtering process. This kinetically assisted potential sputtering mechanism has been identified to be present for ether insulating surfaces as well. [less ▲] Detailed reference viewed: 249 (0 UL) Vertical incidence of slow Ne10+ ions on an LiF surface: Suppression of the trampoline effectWirtz, Ludger ; ; et alin Nuclear Instruments and Methods in Physics Research. Section B, Beam Interactions with Materials and Atoms (2001), 182 We present a Monte Carlo simulation of the neutralization of a slow Ne10+ ion in vertical incidence on an LiF(100) surface. The rates for resonant electron transfer between surface F- ions and the ... [more ▼] We present a Monte Carlo simulation of the neutralization of a slow Ne10+ ion in vertical incidence on an LiF(100) surface. The rates for resonant electron transfer between surface F- ions and the projectile are calculated using a classical trajectory Monte Carlo simulation, We investigate the influence of the hole mobility on the neutralization sequence. It is shown that backscattering above the surface due to the local positive charge up of the surface ("trampoline effect") does not take place. (C) 2001 Elsevier Science B.V. All rights reserved. [less ▲] Detailed reference viewed: 187 (1 UL) Observation of a threshold in potential sputtering of LiF surfaces; ; Wirtz, Ludger et alin Nuclear Instruments and Methods in Physics Research. Section B, Beam Interactions with Materials and Atoms (2000), 164 A quartz-crystal microbalance technique is used for measuring total sputtering yields for LiF under impact of slow (20 eV, 100 eV, 500 eV and 1000 eV kinetic energy) singly and doubly charged ions. At low ... [more ▼] A quartz-crystal microbalance technique is used for measuring total sputtering yields for LiF under impact of slow (20 eV, 100 eV, 500 eV and 1000 eV kinetic energy) singly and doubly charged ions. At low kinetic energies (less than or equal to 100 eV) potential sputtering (PS) (i.e., sputtering due to the projectiles potential energy) clearly dominates over kinetically induced sputtering. New insight into the mechanisms for PS is gained by determining the minimum potential energy necessary to induce PS. The measured potential energy threshold at around 10 eV provides evidence that PS can already be induced by the production of cold holes in the valence band of LiF via resonant neutralisation. (C) 2000 Elsevier Science B.V. All rights reserved. [less ▲] Detailed reference viewed: 222 (1 UL) Modular recursive Green's function method for ballistic quantum transport; ; Wirtz, Ludger et alin Physical Review. B (2000), 62(3), 1950-1960 A modification of the standard recursive Green's function method for quantum transport through microstructures is presented which is based on the decomposition into separable substructures. The Green's ... [more ▼] A modification of the standard recursive Green's function method for quantum transport through microstructures is presented which is based on the decomposition into separable substructures. The Green's functions for these modules are joined by discretized Dyson equations. Nonseparable structures can thereby be calculated with the help of a few recursions with high accuracy. We apply this method to the calculation of ballistic quantum transport through a circular and stadium-shaped quantum dot for high mode numbers to test semi-classical predictions in detail. Among other results we find the breakdown of the semiclassical approximation for long path lengths which is due to the spreading of wave packets in the cavity. [less ▲] Detailed reference viewed: 411 (1 UL) Curve-crossing analysis for potential sputtering of insulatorsWirtz, Ludger ; ; et alin Surface Science (2000), 451(1-3), 197-202 We develop a theoretical model for the recently observed threshold for potential sputtering of LiF by slow singly and doubly charged ions. The threshold coincides with the potential energy to create a ... [more ▼] We develop a theoretical model for the recently observed threshold for potential sputtering of LiF by slow singly and doubly charged ions. The threshold coincides with the potential energy to create a cold hole in the valence band of LiF by resonant neutralization. We calculate the level shift of the incident ion and the deformation of the valence band under the influence of the projectile. Resonant neutralization becomes possible for ions with recombination energies larger than 10 eV in agreement with the experimental findings. (C) 2000 Elsevier Science B.V. All rights reserved. [less ▲] Detailed reference viewed: 194 (0 UL) Charge-state evolution of highly charged ions transmitted through microcapillaries; Wirtz, Ludger ; et alin Physical Review. A (2000), 61(2), The charge-state evolution of highly charged ions transmitted through microcapillaries is studied theoretically by a classical trajectory Monte Carlo simulation.: The interaction of highly charged ions ... [more ▼] The charge-state evolution of highly charged ions transmitted through microcapillaries is studied theoretically by a classical trajectory Monte Carlo simulation.: The interaction of highly charged ions with the internal surface of the capillary is treated within the framework of dielectric response theory. We analyze the distance of closest approach and the angular distributions of the highly charged ions at the exit of the microcapillary. We find the charge-state fraction of transmitted N6+ projectiles, in: good agreement with first measurements. Moreover, our calculations indicate that grazing collisions with the microcapillary surface hold the promise of direct observation of charge transfer and hollow-atom formation at a large distance from the surface. [less ▲] Detailed reference viewed: 254 (8 UL) Gauge-invariant theory for semiclassical magnetotransport through ballistic microstructuresWirtz, Ludger ; ; in Physical Review. B (1999), 59(4), 2956-2967 Within the semiclassical theory of magnetotransport through ballistic cavities, fluctuations in the transmission amplitude and in the conductance originate from the Aharonov-Bohm phase of directed areas ... [more ▼] Within the semiclassical theory of magnetotransport through ballistic cavities, fluctuations in the transmission amplitude and in the conductance originate from the Aharonov-Bohm phase of directed areas. We formulate the semiclassical transmission amplitude in gauge-invariant form. The gauge invariant phases can be visualized in terms of areas enclosed by classical paths, which consist of the real path connecting the entrance point to the exit point and a virtual path leading back to the entrance point. We implement this method on different levels of a semiclassical description of magnetotransport with applications to magnetoconductance fluctuations and correlations. The validity of the semiclassical theories is analyzed. [S0163-1829(99)10903-2]. [less ▲] Detailed reference viewed: 394 (1 UL)![]() Interaction of highly charged ions with microcapillaries; Wirtz, Ludger ; in PHYSICA SCRIPTA (1999), T80B The transmission of highly charged ions (HCI) through microcapillaries is investigated. The interaction of an HCI with the internal surface of the capillary is described in terms of a classical image ... [more ▼] The transmission of highly charged ions (HCI) through microcapillaries is investigated. The interaction of an HCI with the internal surface of the capillary is described in terms of a classical image potential. For Neq+ projectiles transmitted through a Ni capillary the impact parameter distribution and angular distribution of ions leaving the microcapillary is determined. We consider both a narrowly focussed and a dispersive incident beam relative to the acceptance angle of the capillary. Our results are compared with recent experiments. [less ▲] Detailed reference viewed: 158 (5 UL) Threshold for potential sputtering of LiF; ; et al in Physical Review Letters (1999), 83(19), 3948-3951 We have measured total sputtering yields for impact of slow (less than or equal to 100 eV) singly and doubly charged ions on LiF. The minimum potential energy necessary to induce potential sputtering (PS ... [more ▼] We have measured total sputtering yields for impact of slow (less than or equal to 100 eV) singly and doubly charged ions on LiF. The minimum potential energy necessary to induce potential sputtering (PS) from UF was determined to be about 10 eV. This threshold coincides with the energy necessary to produce a cold hole in the valence band of LiF by resonant neutralization. This allows the first unambiguous identification of PS induced by cold holes. Further stepwise increase of the sputtering yield with higher projectile potential energies provides evidence for additional defect-mediated sputtering mechanisms operative in alkali halides. [less ▲] Detailed reference viewed: 173 (0 UL)![]() Interaction of highly charged ions with microcapillaries; Wirtz, Ludger ; in Nuclear Instruments and Methods in Physics Research. Section B, Beam Interactions with Materials and Atoms (1999), 154(1-4), 307-311 We analyze the transmission of highly charged ions (HCI) through microcapillaries. The interaction of an HCI with the interval surface of the capillary is treated within the framework of linear response ... [more ▼] We analyze the transmission of highly charged ions (HCI) through microcapillaries. The interaction of an HCI with the interval surface of the capillary is treated within the framework of linear response. In the limiting case of an ideal conducting cylindrical surface, the interaction reduces to a classical image potential. For Neq+ projectiles transmitting through a Ni capillary calculations for the impact parameter distribution and angular distribution of hollow atoms are presented. We find the fraction of transmitted projectiles which are partially neutralized in good agreement with recent experiments. (C) 1999 Elsevier Science B.V. All rights reserved. [less ▲] Detailed reference viewed: 178 (1 UL) Oscillations in the magnetoconductance autocorrelation function for ballistic microstructures; Wirtz, Ludger ; et alin Physical Review. B, Condensed Matter (1998), 57(16), 9875-9878 We present a comparison between experiment and theory for the magnetoconductance autocorrelation function C(Delta B) for transport through a stadium-shaped ballistic microstructure. The correlation ... [more ▼] We present a comparison between experiment and theory for the magnetoconductance autocorrelation function C(Delta B) for transport through a stadium-shaped ballistic microstructure. The correlation function displays damped oscillations which can be traced to the quantum interference between bundles of short trajectories. We present two different semiclassical calculations applicable for large and small mode numbers of the quantum wire, respectively. Good agreement is found with experimental data taken at relatively low mode numbers. [S0163-1829(98)03316-5]. [less ▲] Detailed reference viewed: 212 (1 UL)![]() Geometry-dependent scattering through ballistic microstructures: Semiclassical theory beyond the stationary-phase approximationWirtz, Ludger ; ; in Physical Review. B (1997), 56(12), 7589-7597 The conductance of a ballistic microstructure shows strong fluctuations as a function of the Fermi wave number. We present a semiclassical-theory that describes these fluctuations in terms of bundles of ... [more ▼] The conductance of a ballistic microstructure shows strong fluctuations as a function of the Fermi wave number. We present a semiclassical-theory that describes these fluctuations in terms of bundles of short trajectories. These trajectories provide the dominant contribution to electron transport through a weakly open microstructure. For the coupling between the quantum wires and the cavity, contributions beyond the stationary phase approximation are taken into account giving rise to diffraction effects. A comparison with full quantum calculations for st rectangular billiard is made. The peak positions of the power spectrum agree very well between the quantum and semiclassical theories. Numerical evidence is found for the breakdown of the semiclassical approximation for long paths. A simple explanation in terms of the dispersion of the semiclassical wave packet in the interior of the cavity is proposed. [less ▲] Detailed reference viewed: 389 (4 UL) |
||